By Andrew Martins, Brian Mariampillai, Mark Lautens (auth.), Jin-Quan Yu, Zhangjie Shi (eds.)

ISBN-10: 3642123554

ISBN-13: 9783642123559

Table of Contents - Synthesis within the Key of Catellani: Norbornene-Mediated ortho C–H Functionalization - Mechanistic issues within the improvement and Use of Azine, Diazine and Azole N-Oxides in Palladium-Catalyzed Direct Arylation - Palladium and Copper Catalysis in Regioselective, Intermolecular Coupling of C–H and C–Hal Bonds - Pd-Catalyzed C–H Bond Functionalization at the Indole and Pyrrole Nucleus - distant C–H Activation through Through-Space Palladium and Rhodium Migrations - Palladium-Catalyzed Aryl–Aryl Bond Formation via Double C–H Activation - Palladium-Catalyzed Allylic C–H Bond Functionalization of Olefins - Ruthenium-Catalyzed Direct Arylations via C–H Bond Cleavages - Rhodium-Catalyzed C–H Bond Arylationof Arenes - Cross-Dehydrogenative Coupling Reactions of sp3-Hybridized C–H Bonds - Functionalization of Carbon–Hydrogen Bonds via Transition steel Carbenoid Insertion - Metal-Catalyzed Oxidations of C–H to C–N Bonds

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1 Synthetic Considerations . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2 Reactivity with Azine and Diazine N-Oxides . . . . . . . . . . . . . . . . . . . . . 3 Regioselectivity with Nonsymmetrical Azine Substrates . . . . . . . . . . . . . . . 4 Azole N-Oxides . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5 Methods for N-Oxide Deoxygenation .

3 Regioselectivity with Nonsymmetrical Azine Substrates . . . . . . . . . . . . . . . 4 Azole N-Oxides . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5 Methods for N-Oxide Deoxygenation . . . . . . . . . . . . . . . . . . . . . . . . . 49 4 Applications in Medicinal Chemistry . . . . . . . . . . . . . . . . . . . . . . . . . . . 51 5 Mechanistic Considerations .

1 Synthetic Considerations . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2 Reactivity with Azine and Diazine N-Oxides . . . . . . . . . . . . . . . . . . . . . 3 Regioselectivity with Nonsymmetrical Azine Substrates . . . . . . . . . . . . . . . 4 Azole N-Oxides . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5 Methods for N-Oxide Deoxygenation .

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C-H Activation by Andrew Martins, Brian Mariampillai, Mark Lautens (auth.), Jin-Quan Yu, Zhangjie Shi (eds.)


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